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Reaction Mechanisms of the Methylation of Ethene with Methanol and Dimethyl Ether over H-ZSM-5: An ONIOM Study

✍ Scribed by Maihom, T.; Boekfa, B.; Sirijaraensre, J.; Nanok, T.; Probst, M.; Limtrakul, J.

Book ID
121453915
Publisher
American Chemical Society
Year
2009
Tongue
English
Weight
437 KB
Volume
113
Category
Article
ISSN
1932-7447

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Methylation of toluene (in one case benzene) with methanol has been investigated over four dierent zeolites: Small and large crystal ZSM-5, dealuminated mordenite and zeolite beta. The feed ratio methanol/arene was varied over a wide range, mostly b1, using nitrogen or helium as carrier gas. A rathe