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Raman scattering study of the orientational dynamics of the methyl bromide

✍ Scribed by A. Kocot; R. Wrzalik

Publisher
Elsevier Science
Year
1996
Tongue
English
Weight
365 KB
Volume
69
Category
Article
ISSN
0167-7322

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✦ Synopsis

Raman band shapes of the v3 vibration in methyl bromide have been studied in the temperature range 183 K to 333 K. The isotropic and anisotropic part of the band were determined and then used to calculate spectral density of the rotational contribution. The integrated spectral density of the rotational contribution has been found to satisfy the second moment criterion. Both rotational correlation function and angular velocity correlation function have been determined and analysed.

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The polarization-resolved resonance hyper-Raman (RHR) scattering of CHJ vapor is observed as blue mcident radiation is tuned through two-photon resonance with the origin absorption band ofthe predissociative c+x Rydberg transition in the WV ( 183-175 nm). These results demonstrate the ability of thi