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Quasiclassical trajectory study of the rotational distribution for the O+NO(v = 0) fundamental vibrational excitation

✍ Scribed by B. R. L. Galvão; J. A. Corzo-Espinoza; P. J. S. B. Caridade; A. J. C. Varandas


Publisher
John Wiley and Sons
Year
2011
Tongue
English
Weight
146 KB
Volume
43
Category
Article
ISSN
0538-8066

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✦ Synopsis


Abstract

Quasiclassical trajectories have been run to study the fundamental one‐quantum vibrational transition formed from collisions of ground‐state nitric oxide with atomic oxygen at temperatures of 500, 750, and 1000 K. Two adiabatic potential energy surfaces of different symmetry (^2^A′ and ^2^A″ of NO~2~) have been utilized. The rate constant for the title process is given along with the rotational distributions, and the results shown to corroborate previous atmospheric models that describe the nascent state by a Maxwell–Boltzmann distribution at the local temperature. © 2011 Wiley Peiodicals, Inc. Int J Chem Kinet 43: 345–352, 2011