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Quadrupole Transitions in CF3Br Investigated by Two-Dimensional Fourier Transform Spectroscopy in the Microwave-Radiofrequency Range

✍ Scribed by H. Harder; H.W. Nicolaisen; H. Dreizler; H. Mader


Publisher
Elsevier Science
Year
1993
Tongue
English
Weight
333 KB
Volume
160
Category
Article
ISSN
0022-2852

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✦ Synopsis


"Pure" quadrupole transitions have been observed in (\mathrm{CF}{3}{ }^{79} \mathrm{Br}) and (\mathrm{CF}{3}{ }^{81} \mathrm{Br}) using the technique of two-dimensional Fourier transform spectroscopy in the microwave and radiofrequency range. We observed transitions for (J=4,5,6) and (K=1, \ldots, 5) in the ground vibrational state for both isotopomers and determined the quadrupole coupling constant ({ }^{Q} Q q_{0}), its rotational dependencies (\bar{\chi}{\kappa}) and (\chi{d}), and the spin-rotation constants (C_{N}) and (C_{\kappa}). For (\mathrm{CF}_{3}{ }^{81} \mathrm{Br}) the rotational dependence (\bar{x}), has also heen determined. 1993 Academic Press. Inc