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Pure rotational transitions of silver chloride prepared in an electric discharge, observed with a cavity microwave Fourier-transform spectometer

✍ Scribed by C. Styger; M.C.L. Gerry

Publisher: Elsevier Science
Year: 1992
Tongue: English
Weight: 274 KB
Volume: 188
Category: Article
ISSN: 0009-2614
DOI: 10.1016/0009-2614(92)90011-b

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✦ Synopsis

Pure rotational transitions of silver chloride generated in an electric discharge have been observed using a cavity microwave Fourier-transform spectrometer. This is the first report of the successful use of this method to generate a metal compound for microwave spectroscopy. The high resolution of the instrument has permitted an improvement of two orders of magnitude in the precision of the 35C1 nuclear quadrupole coupling constants.

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Rotational transitions of \({ }^{28} \mathrm{SiF}_{2}\) and four isotopomers of \(\mathrm{GeF}_{2}\) have been investigated using a cavity pulsed microwave Fourier transform spectrometer. Both molecules were prepared in electric discharges, in \(\mathrm{SiF}_{4}\) and \(\mathrm{GeF}_{4}\), respectiv