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Properties of strong hydrogen-bonded systems. II. Ab initioSCF-MO study of the hydrogen bond between nitric acid and ammonia

✍ Scribed by Z. Latajka; M. M. Szczçśniak; H. Ratajczak; W. J. Orville-Thomas


Publisher
John Wiley and Sons
Year
1980
Tongue
English
Weight
185 KB
Volume
1
Category
Article
ISSN
0192-8651

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✦ Synopsis


Abstract

The hydrogen‐bonded complex between nitric acid and ammonia molecules has been studied by the ab initio molecular orbital method using the 4‐31G basis set. The calculated interaction energy for the complex (Δ__E__ = −91.4 kJ mole^−1^) indicates that one is dealing with the strongest “nonionic” H‐bonded complex considered hitherto by theoretical methods. Other properties of the hydrogen‐bonded complex such as geometrical parameters, dipole moment, amount of charge transfer, and stretching force constants of the OH and (OH)… N bonds are calculated and discussed.