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Preparative Asymmetric Reduction of 3-Ketobutyrate and -valerate by Suspended Cells of Thermophilic Bacteria (Thermoanaerobium brockii) in Ordinary Laboratory Equipment

✍ Scribed by Dieter Seebach; Fabio Giovannini; Bernd Lamatsch


Publisher
John Wiley and Sons
Year
1985
Tongue
German
Weight
212 KB
Volume
68
Category
Article
ISSN
0018-019X

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✦ Synopsis


Abstract

The thermophilic and anaerobic bacteria specified in the title are isolated on a 0.8 kg scale by tangential flow filtration and centrifugation from a 300‐1 bioreactor. The microorganisms are stored in a freezer (−20°) and used, analogously to baker's yeast, for asymmetric reductions. Thus, ethyl 3‐ketovalerate (4.3) g/1 (H~2~O) is converted in 40% yield to (S)‐3‐hydroxyvalerate (6), with an enantiomeric excess of 93% (24 h at 72°).