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Preparation of 14C-labeled 8,9-didehydro-6,8-dimethyl-2-methylthioergoline mesylate, a dopamine antagonist potentially useful in the treatment of schizophrenia

✍ Scribed by William J. Wheeler


Publisher
John Wiley and Sons
Year
1988
Tongue
French
Weight
381 KB
Volume
25
Category
Article
ISSN
0022-2135

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✦ Synopsis


We have prepared 14C-labeled 8,9--6,8-dimethy1-2-methylthioergoline mesylate (LY 170542), a U e antagonist potentially useful as an anti-psychotic. The 14C-label was introduced via a novel application of the Wittig reaction on 1-(4'-toluene-sulfonyl) -8,9-didehydr&6-meth 1 lysergene by lithiudammonia at -33OC. The 17-[14Cl-agroclavine thus prepared was converted into 17-[ 14C]-LY 170542 by reaction with methanesulfenyl chloridelmethanesulfonic acid ergolin-8-one and subsequent reduction of 1-(4'-toluenesulfonyl)-17-[ ? -