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Polyaza[n]paracyclophanes as synthetic models of Zn containing enzymes. The role of a non coordinated nitrogen atom in the proximity of the metal

✍ Scribed by Belen Altava; M.Isabel Burguete; Santiago V. Luis; Juan F. Miravet; Enrique García-España; Victor Marcelino; Conxa Soriano


Book ID
104207683
Publisher
Elsevier Science
Year
1997
Tongue
French
Weight
657 KB
Volume
53
Category
Article
ISSN
0040-4020

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✦ Synopsis


2,6,

9,

paracyclophane (3, B323) represents a simple model for Zn containing enzymes like HCAII which possess additional reactive groups in the l~roximity of the metal center. The Zn2÷.3 complex shows notable catalytic activity for the hydrolysis of p-nitrophenyl acetate Structural modifications of 3 which affect to the non coordinated nitrogen atom greatly modify the catalytic activity of the receptor.