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Polarographic behaviour of hansa yellow- like dyes. Reduction mechanism and substituent effects

✍ Scribed by Ahmad S. Shawall; Bashier A. Abdel Nabey; Cyril Párkányi


Publisher
Elsevier Science
Year
1980
Tongue
English
Weight
458 KB
Volume
25
Category
Article
ISSN
0013-4686

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✦ Synopsis


~Theelectroreduction ofa series of 3-phenyl-2Jdioxopropionanilide 2-arylhydrazones (III) on the dropping mercury electrode (dme) was investigated in eihanolic B&ton-Robinson buffers. In each case, the polarographic curves showed two waves, A and B, corresponding to a four-and a two-electron process, respectively. The E ,,1 valuea for the wave A at pH 8.0 were shown to be a linear function of the Hammctt substituent constant 6; -(E,,,),(V) = 0.982 + 0.1450 (r = 0.989). A mechanism for the polarographic reduction of III is proposed.