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Polarization Measurements of the Resonant Multiphoton Ionization Spectrum of the 3s Rydberg States of Monomethylpyridines

✍ Scribed by C. Kosmidis; A. Bolovinos; P. Tsekeris

Publisher
Elsevier Science
Year
1993
Tongue
English
Weight
271 KB
Volume
160
Category
Article
ISSN
0022-2852

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✦ Synopsis

The circular to linear polarization ratio for the two-photon excitation of the (3 s) Rydberg states of monomethylpyridines has been measured by (2+1) resonant MPI spectroscopy in a static cell. The symmetry of the Rydberg vibrational bands is deduced and the results from the (0-0) transition suggest that the highest occupied MO of 4 -methylpyridine is an (n) MO, while that for 2- and 3methylpyridines is a (\pi)-type one. 1993 Academic Press. Inc.

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