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pH/Thermosensitive Hydrogels Formed at Low pH by a PMMA-PAA-P2VP-PAA-PMMA Pentablock Terpolymer

✍ Scribed by Nikoletta Stavrouli; Ilias Katsampas; Sotirios Aggelopoulos; Constantinos Tsitsilianis


Book ID
102497310
Publisher
John Wiley and Sons
Year
2008
Tongue
English
Weight
215 KB
Volume
29
Category
Article
ISSN
1022-1336

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✦ Synopsis


Abstract

A poly(methyl methacrylate)‐block‐poly(acrylic acid)‐block‐poly(2‐vinyl pyridine)‐block‐poly(acrylic acid)‐block‐poly(methyl methacrylate) (PMMA‐PAA‐P2VP‐PAA‐PMMA), pentablock terpolymer has been synthesized by anionic polymerization with sequential addition of monomers and studied in aqueous media at low pH. The system exhibits combined properties and adopts the behavior of ‘telechelic’ polyelectrolytes and that of double hydrophilic polyampholytes. This complex behavior leads to the pentablock terpolymer forming a pH and temperature sensitive reversible hydrogel at very low polymer concentration.

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