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Ph[PhC(O)NH]2PNC(O)Ph: a new mesomeric stabilized azaylide. Synthesis, crystal structure and IR spectroscopic results

✍ Scribed by T. Saplinova; L. Jäger; A. Kolbe; C. Wagner


Publisher
Elsevier Science
Year
2004
Tongue
English
Weight
167 KB
Volume
690
Category
Article
ISSN
0022-2860

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✦ Synopsis


The structure of Ph[PhC(O)NH] 2 PyNC(O)Ph (2) in solid state and in solution is discussed on the basis of a crystal structure analysis and IR and Raman spectra. In crystalline state 2 forms dimers which are associated via two pairs of bifurcated (N-H) 2 • • •OyC hydrogen bonds. The spectroscopic data are in good agreement with the crystallographic results with respect to the hydrogen bonding and they suggest that 2 also in solution is associated.