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Photoinduced desorption in NO/Pt: a time-dependent quantum mechanical study

✍ Scribed by N. Chakrabarti; V. Balasubramanian; N. Sathyamurthy; J.W. Gadzuk

Publisher: Elsevier Science
Year: 1995
Tongue: English
Weight: 604 KB
Volume: 242
Category: Article
ISSN: 0009-2614
DOI: 10.1016/0009-2614(95)00749-t

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✦ Synopsis

We have carried out a TDQM study of photoinduced desorption in NO/Pt by involving hot electron transfer and allowing different residence times (ZR) on the excited state potential-energy surface. The desorption probabifity (P~) is dependent on ~'g, but it is clear from the results that the substantial P~ can be accounted for by assuming TR is in the range 20-60 fs. The study also accounts for vibrational excitation in the desorbed NO.

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