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Photodissociation of CH4+ via ion cyclotron resonance

โœ Scribed by M. Riggin; R.C. Dunbar

Publisher
Elsevier Science
Year
1975
Tongue
English
Weight
462 KB
Volume
31
Category
Article
ISSN
0009-2614

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โœฆ Synopsis

The molecular methane ion C*q was observed to dissociate to the methyl cation and a hydrogen atom upon irradiation with white li&t from a 2.5 K'T' xenon arc lamp. The maximum photodissociation CIOSS section was estimated as 3 X LO-l9 cm' at 3350 A and a spectrum was obtained.

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Close coupling ~lculakms for the photodissociation cross sections of CH++ hv\* C?(\*P) + H(\*S) exhibit near threshold peaks not ascribable only to quasi-bound 1eveLF in the A 'It potential. Our ckulations demonstrate the importance of non-adiabatic transitions and thereby suggest the necewty to rev