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Phase Separation and Organisation of Colloidal Spheres Suspended in Sheared Lyotropic Liquid-Crystalline Polymers

✍ Scribed by Shanju Zhang; Eugene M. Terentjev; Athene M. Donald


Publisher
John Wiley and Sons
Year
2005
Tongue
English
Weight
219 KB
Volume
26
Category
Article
ISSN
1022-1336

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✦ Synopsis


Abstract

Summary: Organisation behaviours of spherical particles suspended in sheared, lyotropic, liquid‐crystalline polymer solutions have been investigated using polarizing optical microscopy. We find that in a nematic phase the particles phase separate and adopt anisotropic chain‐like structures along the director. An earring defect is observed around a single particle whereas a cross or strings defect between neighbouring particles is found to serve as a repulsive barrier to prevent the particles from contacting each other. A theoretical analysis is presented to explain this new phenomenon.

An optical micrograph of 0.01 wt.‐% glass spheres suspended in a nematic solution of 40 wt.‐% ethyl cellulose in chloroform under an external shear force.

magnified imageAn optical micrograph of 0.01 wt.‐% glass spheres suspended in a nematic solution of 40 wt.‐% ethyl cellulose in chloroform under an external shear force.