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pH-Responsive PEG-Poly(β-amino ester) Block Copolymer Micelles with a Sharp Transition

✍ Scribed by Min Sang Kim; Su Jong Hwang; Jong Kwon Han; Eun Kyung Choi; Heon Joo Park; Jin Seok Kim; Doo Sung Lee


Publisher
John Wiley and Sons
Year
2006
Tongue
English
Weight
132 KB
Volume
27
Category
Article
ISSN
1022-1336

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✦ Synopsis


Abstract

Summary: A pH‐sensitive block copolymer is synthesized by step polymerization and its pH‐sensitive micellization‐demicellization behavior is studied. This polymer has a hydrophilic MPEG (shell) and hydrophobic but pH‐sensitive poly(β‐amino ester) (core), which can form a self‐assembled micelle. As confirmed by fluorescence spectroscopy and dynamic light scattering (DLS), this polymer shows a sharp pH‐sensitive micellization‐demicellization behavior. It is confirmed that the pH sensitivity is affected by the molecular weight ratio between the MPEG and poly(β‐amino ester).

Plots of the intensity ratio I~337~/I~334~ (from pyrene excitation spectra): a) vs. pH for copolymer samples and b) vs. log (concentration) for M1.

magnified imagePlots of the intensity ratio I~337~/I~334~ (from pyrene excitation spectra): a) vs. pH for copolymer samples and b) vs. log (concentration) for M1.