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Partial Protection against Botulinum B Neurotoxin-Induced Blocking of Exocytosis by a Potent Inhibitor of Its Metallopeptidase Activity

✍ Scribed by Christine Anne; Serge Turcaud; Armand G. S. Blommaert; François Darchen; Eric A. Johnson; Bernard P. Roques


Book ID
101816119
Publisher
John Wiley and Sons
Year
2005
Tongue
English
Weight
107 KB
Volume
6
Category
Article
ISSN
1439-4227

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✦ Synopsis


Abstract

Clostridium botulinum neurotoxins (BoNTs) cause botulism, which is characterized by a flaccid paralysis, through inhibition of acetylcholine release by peripheral cholinergic nerve terminals. This is due to the zinc metallopeptidase activity of the neurotoxin, cleaving one component (synaptobrevin for BoNT/B) of the exocytosis machinery. Yet, there are no specific agents able to control the peptidase‐related effects of BoNT/B. We recently developed the first compounds to inhibit this enzymatic activity in the nanomolar range. Here we report that two of our best inhibitors prevent the BoNT/B‐induced cleavage of native synaptobrevin on synaptic vesicles, and partially inhibit the suppression of [^3^H]noradrenaline release from synaptosomes that is caused by BoNT/B. These results were obtained at micromolar concentrations, consistent with the measured inhibitory potency of these inhibitors on the native toxin. These compounds provide a new way to possibly prevent and/or to control the neurotoxin effects of botulinum.