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Palladium(II)-catalyzed dicarboxymethylation of chiral allylic alcohols: chirality transfer affording optically active diesters containing three contiguous chiral centers

✍ Scribed by Othman Hamed; Patrick M. Henry; Daniel P. Becker


Book ID
104097778
Publisher
Elsevier Science
Year
2010
Tongue
French
Weight
680 KB
Volume
51
Category
Article
ISSN
0040-4039

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✦ Synopsis


This manuscript describes the extension of Stille's palladium-catalyzed olefin dicarbonylation reaction to chiral allylic alcohols with chirality transfer to afford the corresponding chiral alcohol functionalized with bis-carbomethoxy esters, containing three contiguous chiral centers, in good to excellent diastereoselectivities (78-98%).