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Palladium-based electrodes: A way to reduce platinum content in polymer electrolyte membrane fuel cells

✍ Scribed by Ermete Antolini; Sabrina C. Zignani; Sydney F. Santos; Ernesto R. Gonzalez


Publisher
Elsevier Science
Year
2011
Tongue
English
Weight
955 KB
Volume
56
Category
Article
ISSN
0013-4686

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✦ Synopsis


To decrease the Pt content, a polymer electrolyte membrane fuel cell (PEMFC) was formed using a carbon supported Pd 96 Pt 4 catalyst as the anode material, and a carbon supported Pd 49 Pt 47 Co 4 catalyst as the cathode material. The as-obtained Pd-based PEMFC with an overall Pd:Pt:Co atomic composition of electrodes (anode + cathode) = 72:26:2 exhibited a performance not too far from that of the fuel cell with the conventional 100% Pt electrodes. With a Pt content of 35 wt% of that of the cell with full Pt electrodes, at a current density of 1 A cm -2 the performance loss of the cell with the Pd-based catalysts was only 11%, with 6% ascribed to the anode catalyst and 5% to the cathode catalyst. The maximum power density of the Pd-based cell was 76% of that of the cell with Pt catalysts.