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On the spectroscopic behaviour of o-bis(o-phenylendiimido) nickel

✍ Scribed by F. Lelj; A. Rosa; G.P. Ricciardi; M. Casarin; P.L. Cristinziano; G. Morelli

Book ID: 103029734
Publisher: Elsevier Science
Year: 1989
Tongue: English
Weight: 303 KB
Volume: 160
Category: Article
ISSN: 0009-2614
DOI: 10.1016/0009-2614(89)87551-7

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✦ Synopsis

The ground state electronic structure of bis( o-phenylendiimido)Ni has been thoroughly investigated using the fast principle discrete-variational local exchange ( DV-Xa! ) technique, according to the SCC (self-consistent charge) and SCM (self-consistent multicenter-multipolar)

approximations.

New UV-visible and near-IR absorption experiments, using solvents with different donor power, are presented. Electronic excitations, computed according to Slater's transition state procedure, are compared with spectra recorded in CH&. The reported results shed new light on the origin of the spectroscopic behaviour of the title complex.

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