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On the Spectral Similarities between 1,2,6,7-Tetracyano-3,5-dihydro-3,5-diiminopyrrolizinato Complexes and Phthalocyanines – X-ray Crystal and Molecular Structure of Two Mixed Monopyrrolizinato Nickel(II) Complexes with the 2,4-tert-Butylacetylacetonide Ligand

✍ Scribed by Alberto Flamini; Vincenzo Fares; Augusto Pifferi


Publisher
John Wiley and Sons
Year
2000
Tongue
English
Weight
414 KB
Volume
2000
Category
Article
ISSN
1434-1948

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✦ Synopsis


Complexes of Ni II , Cu II , Zn II , and Co III containing the 1,2,6,7tetracyano-3,5-dihydro-3,5-diiminopyrrolizinide (L) and the 2,4-tert-butylacetylacetonide (DPM) ligands have been synthesized and characterized. The absorption optical spectra of these species and of the corresponding ML 2 complexes in coordinating solvents are compared with those of metalphthalocyanines (MPc) and hydrogen-phthalocyanine (H 2 Pc), respectively. The comparison shows a close similarity, especially for the nickel-containing species, in the low-energy spectral region where the first πǞπ* transitions occur (Q band). The Q band position of the pyrrolizinato complexes