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On the Mechanism of the Anionic Oxy-Cope Rearrangement of trans-1,2-Dialkenylcyclobutanols

✍ Scribed by Philippe Maurin; Se-Ho Kim; Sung Yun Cho; Jin Kun Cha

Publisher
John Wiley and Sons
Year
2003
Tongue
English
Weight
133 KB
Volume
42
Category
Article
ISSN
0044-8249

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The 3-aza-Cope rearrangements of 3-azoniahexa-1,5-diene (1), 3-azoniahex-1-ene-5-yne (3), and 3-azahex-1-ene-5-yne (5) were investigated up to the coupled-cluster level, CCSD(T), by using a valence triple-zeta basis set. Activation barriers and geometrical parameters of the transition states are pro