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On the lack of evidence for contact contributions to lanthanide-induced N.M.R. shifts (L.I.S.'s) in aromatic aldehydes: a rigorous error analysis and the isolation of diamagnetic (complexation) shifts.

✍ Scribed by Raymond J Abraham; Derek J Chadwick


Publisher
Elsevier Science
Year
1981
Tongue
French
Weight
256 KB
Volume
22
Category
Article
ISSN
0040-4039

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✦ Synopsis


The adoption of a rigorous error analysis of L.I .S. 's allows the non-pseudo-contact components of the Yb(fod)a induced shifts in benzaldehyde and thiophen-Z-aldehyde to be isolated.

They are largest at the carbonyl carbon and at the ortho and pam carbons and appear to be entirely due to complexation (diamagnetic) shifts. Estimation of these with La (fod)a allows a precise analy-