✦ LIBER ✦

On the Calculation of Resonance Raman Spectra

✍ Scribed by R. Islampour; M. Hayashi; S. H. Lin

Publisher: John Wiley and Sons
Year: 1997
Tongue: English
Weight: 434 KB
Volume: 28
Category: Article
ISSN: 0377-0486
DOI: 10.1002/(sici)1097-4555(199705)28:5<331::aid-jrs101>3.0.co;2-4

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✦ Synopsis

A general formalism for resonance Raman scattering is presented which treats both linear and quadratic electronphoton interactions. The time correlation functions which are involved in resonance Raman scattering both from a single vibronic state and from the initially distributed vibronic states are calculated. The expressions are exact for a displaced-distorted oscillator system at all temperatures. The e †ects of distortions of potential energy surfaces on absorption, resonance Raman excitation proÐles and resonance Raman spectra were also investigated quantitatively.

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