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On the bonding in doubly charged diatomics

✍ Scribed by Jörg Senekowitsch; Stephen ONeil; Wilfried Meyer

Publisher
Springer
Year
1992
Tongue
English
Weight
547 KB
Volume
84
Category
Article
ISSN
1432-2234

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📜 SIMILAR VOLUMES

On the formation of doubly charged ions
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## Abstract The observation of doubly charged ions in field ionization with blade or wire emitters does not in itself indicate that high excitation energies (≥ 17 eV) are accessible through gas phase ionization with such emitters.

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We investigate, by means of ab initio calculations, the strength of electron correlations within covalent bonds: the first-row homonuclear diatomics serve as test cases. As an appropriate measure of the correlation strength, we introduce the reduction of the mean-square deviations of the electronic