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Observation of highly charged sodium clusters

✍ Scribed by Näher, U.; Göhlich, H.; Lange, T.; Martin, T. P.

Book ID
121333976
Publisher
The American Physical Society
Year
1992
Tongue
English
Weight
362 KB
Volume
68
Category
Article
ISSN
0031-9007

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Small, highly charged sodium clusters have been produced by multi-step ionization of large clusters followed by evaporative shrinking. The critical size, nc, beyond which Na~ + are stable obeys the approximate relation he= 8z 2. However, significant deviations from constant z2/n¢ are dearly evident.

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Small doubly charged niobium clusters are observed in a molecular beam emerging from a laser vaporization/supersonic expansion source if electron impact ionization is utilized in the expansion region. Doubly charged clusters from n=2 to n= I5 are readily detected. The doubly charged dimer cation has