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Novel One-Step Route for Preparing Amphiphilic Block Copolymers of Styrene and N-Isopropylacrylamide in a Microemulsion

✍ Scribed by Cheng Zheng; Wei-Dong He; Wei-Jun Liu; Jian Li; Jun-Fang Li


Publisher
John Wiley and Sons
Year
2006
Tongue
English
Weight
94 KB
Volume
27
Category
Article
ISSN
1022-1336

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✦ Synopsis


Abstract

Summary: Copolymerizations of St and NIPAM have been carried out through interfacial‐initiated microemulsion polymerization in a frozen state. FT‐IR and NMR spectroscopies confirm the occurrence of copolymerization between the two monomers. DSC analysis shows the existence of two glass transition temperatures of the resultant copolymers. The micellization of the copolymers is investigated by DLS and the temperature‐responsive behavior of the resultant micelles is observed. DSC and DLS results reveal the block feature of the obtained copolymers. Thus amphiphilic poly(styrene‐blockN‐isopropylacrylamide) is prepared by a one‐step interfacial‐initiated microemulsion polymerization.

Hydrodynamic radius of the micellar particles formed by (left), and a typical DSC trace of (right), the poly(styrene‐blockN‐isopropylacrylamide) prepared here.

magnified imageHydrodynamic radius of the micellar particles formed by (left), and a typical DSC trace of (right), the poly(styrene‐blockN‐isopropylacrylamide) prepared here.