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Novel cellulose derivatives. I. Liquid crystal phase formation in tri-O-α-naphthylmethyl cellulose solutions

✍ Scribed by Vipul Davé; Charles E. Frazier; Wolfgang G. Glasser


Publisher
John Wiley and Sons
Year
1993
Tongue
English
Weight
778 KB
Volume
49
Category
Article
ISSN
0021-8995

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✦ Synopsis


Tri-0-a-naphthylmethyl cellulose was prepared by homogeneous phase reaction using SO2diethylamine (DEA) -dimethyl sulfoxide (DMSO) as the solvent system. Observations made by dynamic mechanical spectrometry and by cross-polarized optical microscopy revealed liquid crystalline behavior for the concentrated solutions of tri-0-a-naphthylmethyl cellulose in dimethylacetamide ( DMAc ) . Experimental and calculated (predicted) critical volume fraction of the derivative, Vk, did not show agreement. It is determined that V i is affected by bulky substituents on the cellulose backbone to some extent.