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Non-orthogonal orbitals in MCHF or configuration interaction wave functions

✍ Scribed by A. Hibbert; C. Froese Fischer; M.R. Godefroid


Publisher
Elsevier Science
Year
1988
Tongue
English
Weight
651 KB
Volume
51
Category
Article
ISSN
0010-4655

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✦ Synopsis


The method of calculating interaction matrix elements between multi-configurational wave functions, given by Fano (1965) for orthogonal orbitals, is extended to allow the use of non-orthogonal orbitals. We allow up to two subshells in each configuration function which contain spectator (non-interacting) electrons described by orbitals which are not orthogonal to orbitals in the other configuration function of the matrix element. A discussion of the effects of less restrictive conditions is presented.