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New out-of-plane angle and bond angle internal coordinates and related potential energy functions for molecular mechanics and dynamics simulations

✍ Scribed by Lee, Sang-Ho; Palmo, Kim; Krimm, Samuel


Publisher
John Wiley and Sons
Year
1999
Tongue
English
Weight
315 KB
Volume
20
Category
Article
ISSN
0192-8651

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✦ Synopsis


With currently used definitions of out-of-plane angle and bond angle internal coordinates, Cartesian derivatives have singularities, at "r2 in the former case and in the latter. If either of these occur during molecular mechanics or dynamics simulations, the forces are not well defined. To avoid such difficulties, we provide new out-of-plane and bond angle coordinates and associated potential energy functions that inherently avoid these singularities. The application of these coordinates is illustrated by ab initio calculations on ammonia, water, and carbon dioxide.