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New Nonlinear Optical Materials: Expedient Topotactic Self-Assembly of Acentric Chromophoric Superlattices

✍ Scribed by Dr. Wenbin Lin; Dr. Shlomo Yitzchaik; Weiping Lin; Amit Malik; Mary K. Durbin; Andrew G. Richter; Prof. George K. Wong; Prof. Pulak Dutta; Prof. Tobin J. Marks


Publisher
John Wiley and Sons
Year
1995
Tongue
English
Weight
383 KB
Volume
34
Category
Article
ISSN
0044-8249

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✦ Synopsis


COM MU NlCATlONS

mechanism-specific orbital selection rules. It is demonstrated that the orbital selection rules set stringent structural requirements on the geometries of both the ET-TS and the twin SUB-TS, and determine all of their stereochemical informationstereospecificity. regiospecificity, orientational specificity-and the consequent activation barriers. Thus, the ET-TS is found to possess a robust stereochemistry that follows the maximum bonding principle allowed by the selection rule. The existence of kinetic isotope effects for the ET-TS may help establish or challenge the structured ET-TS presented here, and put it in perspective with the traditional notion of weak bonding in the outer sphere model.["-