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Nanostructural characterization of Y123 and Gd123 with BaZrO3 rods fabricated by pulsed-laser deposition

✍ Scribed by Takeharu Kato; Hirokazu Sasaki; Yuki Gotoh; Yukichi Sasaki; Tsukasa Hirayama; Kazuhiro Takahashi; Masaya Konishi; Hiroyoshi Kobayashi; Akira Ibi; Takemi Muroga; Seiki Miyata; Tomonori Watanabe; Yutaka Yamada; Teruo Izumi; Yuh Shiohara


Publisher
Elsevier Science
Year
2006
Tongue
English
Weight
384 KB
Volume
445-448
Category
Article
ISSN
0921-4534

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✦ Synopsis


Both YBa 2 Cu 3 O 7Àx (Y123) and GdBa 2 Cu 3 O 7Àx (Gd123) layers with BaZrO 3 (BZO) rods were deposited on Hastelloy tapes with textured buffer layers (CeO 2 /Gd 2 Zr 2 O 7 ) using pulsed-laser deposition (PLD). Two volume percent of YSZ-Y123 and 2 vol%YSZ-Gd123 were used as target materials. The critical current density (J c ) values of these layers in a magnetic field parallel to the substrate normal were enhanced compared with those of Y123 layers without BZO rods. In the entire incident angle of magnetic fields, the J c reduction of the Gd123 layer with BZO rods were improved compared to that of the Y123 layer with BZO rods. Transmission electron microscopy was used to characterize the nanostructures of the specimens prepared by both focused ion beam and standard ion milling. The Y123 layer with BZO rods and the Gd123 layer with BZO rods were composed of c-axis oriented grains, in which BZO rods aligned in the [0 0 1] of Y(Gd)123 ware distributed homogeneously. The diameter of the BZO rods was about 5 nm and the rods grew from the CeO 2 interface to the surface. The orientation relationships between Y(Gd)123 and BZO were as follows: (0 0 1)Y(Gd)123// (0 0 1)BZO and (1 0 0)Y(Gd)123//(1 0 0)BZO. In the Gd123 with BZO rods, a high density of stacking faults in the (0 0 1) plane and distorted (0 0 1) planes were found. The formation of the BZO rods in the Y(Gd)123 and a high density of defects with respect to the (0 0 1) plane in the Gd123 were considered to enhance the J c values in high magnetic fields.