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Nachbargruppeneffekte in der Gas-Phase: Intramolekulare Deacetalisierung von Hydroxyacetalen unter den Bedingungen der chemischen Ionisation

✍ Scribed by Stefan Matile; Agnes Janowitz; Sandro Ghirlanda; Annalaura Lorenzi-Riatsch; Albert Horni; Attila Moricz; Stefan Bienz; Norbert Bild; Wolf-Dietrich Woggon; Manfred Hesse


Publisher
John Wiley and Sons
Year
1993
Tongue
German
Weight
298 KB
Volume
76
Category
Article
ISSN
0018-019X

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✦ Synopsis


Neighboring-Group Participation in the Gas Phase: Intramolecular Deacetalization of Hydroxyacetals under the Conditions of Chemical Ionization

Under the conditions of chemical ionization (NH,, isobutane, ND,), hydroxyacetals do not show the expected [M + H]+ signal, but the peak corresponding to the loss of the alcohol component of the acetal. This reaction is dependent on the presence of the OH group in the vicinity of the acetal and on the ring size of the heterocycle being formed. M" is detected to a small extent as a consequence of charge exchange during chemical ionization. ~~ ') *) ')