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n-Type Building Blocks for Organic Electronics: A Homologous Family of Fluorocarbon-Substituted Thiophene Oligomers with High Carrier Mobility

✍ Scribed by A. Facchetti; M. Mushrush; H.E. Katz; T.J. Marks


Publisher
John Wiley and Sons
Year
2003
Tongue
English
Weight
217 KB
Volume
15
Category
Article
ISSN
0935-9648

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✦ Synopsis


A substantial enhancement of thermal stability, volatility, and electron affinity, switching the semiconducting behavior from p‐ to n‐type, is achieved by fluoroalkyl substitution of thiophene oligomers (see Figure). When this novel series is compared with the fluorine‐free analogues, trends in molecular packing, optical absorption, HOMO–LUMO gap, and π–π interactions are found to be strikingly similar.