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N( 4 S) Formation following the 193.3-nm ArF Laser Irradiation of NO and NO 2 and Its Application to Kinetic Studies of N( 4 S) Reactions with NO and NO 2

โœ Scribed by Nakayama, Tomoki; Takahashi, Kenshi; Matsumi, Yutaka; Shibuya, Kazuhiko

Book ID
127232423
Publisher
American Chemical Society
Year
2005
Tongue
English
Weight
81 KB
Volume
109
Category
Article
ISSN
1089-5639

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SCFโ€“Xฮฑโ€“SW calculations have been carried out for SN, S2N2, and S4N4 as well as the analogous oxides NO and N2O2. The electronic charge distribution of the sulfides is remarkably uniform leading to highly polar SN bonds (โˆผS+1/2Nโˆ’1/2) in contrast to the oxides where the NO bonds involve less charge tr