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Multiplicity and stability of oscillatory states in a continuous stirred tank reactor with exothermic consecutive reactions A → B → C

✍ Scribed by Donald S. Cohen; James P. Keener


Publisher
Elsevier Science
Year
1976
Tongue
English
Weight
805 KB
Volume
31
Category
Article
ISSN
0009-2509

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✦ Synopsis


Ah&a&-We study the dimensionless heat and mass balance equatibns describing a continuous stirred tank reactor in which there is occurring consecutive first order exothermic reactions. A~~~ ~ymptotic ~c~ations and muner$g calculations are presentqd for both steady states and oscillatory states. A formal perturbation theory, via multitiie scale techniques, is derived to account for limit cycles in phase space. The theory produces for&as whiih are immediately interpretable phisicafly and from which the stability of @e oscillations is immediately resolved without recourse to further techniques. Fur&em&e, numerical cakulatiot8 via our theory are performed whi& are far cheaper and easiek than a direct numerical search and computation involviug the long time study of the basic different&l equations.


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