Multiplex pure rotational coherent anti-stokes Raman spectroscopy in a molecular beam
✍ Scribed by Nicolaas Bloembergen; Kuei-Hsien Chen; Cheng-Zai Lü; Eric Mazur
- Publisher
- John Wiley and Sons
- Year
- 1990
- Tongue
- English
- Weight
- 586 KB
- Volume
- 21
- Category
- Article
- ISSN
- 0377-0486
No coin nor oath required. For personal study only.
📜 SIMILAR VOLUMES
Reported is the fust observation of saturation broadening in a high-resoiution coherent Raman spectrum of the "2 Qbranch of acetylene The measured saturation broadening of 1050 MHz is significantly greater than the ulculatcd nc Stark broadening of less than 100 MHz.
## Abstract Coherent anti‐Stokes Raman scattering (CARS) spectroscopy of gas‐phase CO~2~ is demonstrated using a single femtosecond (fs) laser beam. A shaped ultrashort laser pulse with a transform‐limited temporal width of ∼7 fs and spectral bandwidth of ∼225 nm (∼3500 cm^−1^) is employed for simu