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More Arrows in the Quiver: New Pathways and Old Problems with Heavy Alkaline Earth Metal Diphenylmethanides

✍ Scribed by Jacob S. Alexander; Karin Ruhlandt-Senge


Publisher
John Wiley and Sons
Year
2004
Tongue
English
Weight
149 KB
Volume
10
Category
Article
ISSN
0947-6539

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✦ Synopsis


Abstract

Progress in the field of σ‐bonded alkaline earth organometallics has been handicapped by numerous complications, such as high reactivity, low solubility, and the limited availability of suitable starting materials. Here we present two synthetic methods, hydrocarbon elimination and desilylation, as alternative routes into this chemistry. A novel barium diphenylmethanide was prepared using these routes delineating that both methods provide a powerful, versatile synthetic access route to an extended library of organometallic alkaline earth derivatives.