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Molecule—surface collision-induced dissociation of internally excited NO2 on MgO(100)

✍ Scribed by H. Ferkel; J.T. Singleton; H. Reisler; C. Wittig

Publisher: Elsevier Science
Year: 1994
Tongue: English
Weight: 548 KB
Volume: 221
Category: Article
ISSN: 0009-2614
DOI: 10.1016/0009-2614(94)00299-1

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✦ Synopsis

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Collision-induced dissociation (CID) of highly excited NOs in the mixed 2A,/2B2 electronic system has been observed for well characterized MgO ( 100) surfaces with parent and product angular resolution at various internal energies. NO state distributions were probed by two-photon, two-frequency ionization, and its yield was found to track the NO2 absorption spectrum, confirming the CID mechanism. The angular dependence of the NO state distribution indicates that CID occurs following direct inelastic scattering rather than trapping-desorption.

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