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Molecular quadrupole moment determinations from measurements of laser wave hyper-Rayleigh scattering by dense fluids

✍ Scribed by J.R. Lalanne; F.B. Martin; S. Kielich


Publisher
Elsevier Science
Year
1975
Tongue
English
Weight
412 KB
Volume
30
Category
Article
ISSN
0009-2614

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✦ Synopsis


Hyper-Rayleigh scattering (second-harmonic scattering, SHS) of laser waves by dense tluids composed ofcentrcsymmetric molecules permits the measurement of the mean-squared value of the internal molecukr electric field !Fi>. In the case of quadrupolar molecules, these measured values can be used to determine the quedrupolc mamcnt of the scattering molecules. NumcricaJ results are given for cyclohexane and fmnsdecahydronaphthdene amounting to 11 and 9.8, respectiveIy, in 10Wz6 esu.