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MM2 study of 20-hydroxy-4,7,13,16-tetraoxa-1,10-diazabicyclo [8,8,3] heneicosane and its formation controlled by hydrogen bonding

✍ Scribed by Ivan Stibor; Petr Holý; Pavel Hobza; Petr Čársky


Publisher
John Wiley and Sons
Year
1990
Tongue
English
Weight
610 KB
Volume
11
Category
Article
ISSN
0192-8651

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✦ Synopsis


A van der Waals-type parameter set has been developed for hydrogen bonding in the MM2(85) force field to reproduce the structures and binding energies of complexes (HzOIz, (CH30H12, H3N . . HzO, H3N . . . HOCH3, (CH313N * HzO, and HCONHz . -. HzO reported in the literature. The MM2(85) force field modified in this way was then applied to the title compound to explain its unexpected stability, unusual properties of its hydroxyl group, and solvent effect on the reaction mechanism in the condensation of Kryptofix 22@ with epichlorohydrine.