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Migration of redundant ethynyl substituents along polycyclic aromatic hydrocarbon peripheries. Consequences for polycyclic aromatic hydrocarbon build up

✍ Scribed by Martin Sarobe; Leonardus W. Jenneskens; Arjan Kleij; Maria Petroutsa


Book ID
104258001
Publisher
Elsevier Science
Year
1997
Tongue
French
Weight
222 KB
Volume
38
Category
Article
ISSN
0040-4039

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✦ Synopsis


The formation of cyclopenta[cd]pyrene (5) and benzo[ghi]fluoranthene (6) upon FVT of 3,9bisethynylphenanthrene (1) and 8-ethynylfluoranthene (2), respectively, suggests that redundant ethynyl substituents, which cannot give five-and/or six-membered ring formation via ethynyl ethylidene carbene equilibration followed by carbene C-H insertion, can migrate along the PAH periphery at high temperatures.