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Microkinetic analysis and mechanism of the water gas shift reaction over copper catalysts

✍ Scribed by Rostam J. Madon; Drew Braden; Shampa Kandoi; Peter Nagel; Manos Mavrikakis; James A. Dumesic

Book ID
113686984
Publisher
Elsevier Science
Year
2011
Tongue
English
Weight
800 KB
Volume
281
Category
Article
ISSN
0021-9517

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A previously developed 13 elementary step microkinetic mechanism for the WGSR on Cu(1 1 1) [Surf. Sci. 512 (2002) 229] is extended by including four new elementary steps. Employing a systematic reaction route analysis, the microkinetic model is further analyzed, simplified and reduced. It is shown t