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Metal Complexes of a Tetraazacyclotetradecane Bearing Highly Fluorinated Tails: New Catalysts for the Oxidation of Hydrocarbons under Fluorous Biphasic Conditions

✍ Scribed by Gianluca Pozzi; Marco Cavazzini; Silvio Quici; Simonetta Fontana


Publisher
Elsevier Science
Year
1997
Tongue
French
Weight
626 KB
Volume
38
Category
Article
ISSN
0040-4039

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✦ Synopsis


Thecommercially availabIemacrocycIetetraszacycIotetradecane (cyclam)has beenconverted into the fluorocarbonsoluble Iigand 1 by N-functionalizationwith RFCH20CH2CH20TS 3, wherein RF is a (per)ffuorooxyalkylenic chain. Upon complexation with 1, transition metal salts can be selectivelysolubilizedin fluorocarbonsthusprovidingnew catalystsfor the oxidativefunctionalizationof hydrocarbonsunderfluorousbiphasic(FB)conditions. 01997 Elsevier ScienceLtd.