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Mediated electron transfer demonstrated with [Ru(BIPY)2Cl poly(4-vinylpyridine)]Cl coated MoSe2 and WSe2 photoanode

✍ Scribed by Otto Haas; N. Müller; H. Gerischer


Publisher
Elsevier Science
Year
1982
Tongue
English
Weight
432 KB
Volume
27
Category
Article
ISSN
0013-4686

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✦ Synopsis


It is shown that at illumina ta! n-MO& and n-WScz electrodes the charge transfer of a hole from the crystal valence baud to certain redox ions in solution is cataiyzed by a [Ru(bipy),CI poly(4+inylpyridine)]Cl covering layer attached at the crystal surface. The coating behaves like a solid redox system taking over the holes from the crystal valence band and passing them to the electrolyte. The oxidized polymer can inicct holes into the valence band of the crystal. Possible applications of this and similar surface coatings