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Mechanism of the Rhodium(III)-Catalyzed Arylation of Imines via C–H Bond Functionalization: Inhibition by Substrate

✍ Scribed by Tauchert, Michael E.; Incarvito, Christopher D.; Rheingold, Arnold L.; Bergman, Robert G.; Ellman, Jonathan A.

Book ID: 118043074
Publisher: American Chemical Society
Year: 2012
Tongue: English
Weight: 667 KB
Volume: 134
Category: Article
ISSN: 0002-7863
DOI: 10.1021/ja211110h

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The catalytic functionalization of unreactive C À H bonds remains one of the major challenges in chemistry. [1] Metal ± boryl systems have been shown to promote stoichiometric [2] and photocatalytic [3] conversion of alkane and arene CÀH bonds into CÀB(OR) 2 groups by using B 2 pin 2 (pin OC-Me 2 CM