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Measurement of the complex second hyperpolarizability of gaseous benzene at 514.5 nm using electric-field-induced second-harmonic generation

✍ Scribed by A. Pantinakis; K.J. Dean; A.D. Buckingham


Publisher
Elsevier Science
Year
1985
Tongue
English
Weight
136 KB
Volume
120
Category
Article
ISSN
0009-2614

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✦ Synopsis


We have measured lhe second hyperpnlariwbility. y. of gaseous benzene nt 514.5 nm with t cw Ar ion laser usin_e the technique of eleclric-fi;ld-induced second-harmonic genrmkn. under periodic phase-matching conditions and by mixing the benzene vnpour with a host gas (Ar or CO:). The use of mixtures allows mcasuremen[ of [he hyperpolariwhilir~ or ~apours of volatile liquids 31 room temperuure and 31 rrcquency regions where the gas under swdy ah.wrbs linearly 3~ the stivond harmonic. Both real and imaginary parts of y xc measured.