Transient methods, such as those with pulse-or stepwise heating, have often been used to measure thermal diffusivity of various materials including layered composite materials. The aim of the present study is to investigate effects of various parameters on the measurement of thermal diffusivity when the transient methods are applied. Mainly a two-layered material in the pulsewise heating method is considered because of its simplicity and usefulness in identifying and determining the effects of the parameters. First, it has been shown that there exists a special condition for determining the thermal diffusivity of a component in the two-layered material whose other relevant thermophysical properties are known. Second, it has been shown that the thickness of the laserbeam absorption layer, which inevitably makes sample material into the twolayered material, may cause a relatively large error when the thermal diffusivity of the base material is high. Finally, it has been derived a definite relation between the apparent thermal diffusivity obtained from the temperature response and the mean thermal diffusivity, which has a physical meaning related to the thermal resistance.