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Mass transfer parameter estimation using optimization technique: Case study in CO2 absorption with chemical reaction

✍ Scribed by Xinsheng Ji; Weerapong Kritpiphat; Ahmed Aboudheir; Paitoon Tontiwachwuthikul


Publisher
John Wiley and Sons
Year
1999
Tongue
English
Weight
453 KB
Volume
77
Category
Article
ISSN
0008-4034

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✦ Synopsis


Abstract

This paper proposes a new approach of applying an optimization technique to simultaneously determine a physical liquid—film mass transfer coefficient (K^o^~L~) and effective interfacial area (a~v~) from a pilot plant data. The mass transfer mechanism of the CO~2~‐NaOH system was modeled using the two‐film theory to represent the behaviors of packed absorbers. The model presents an overall absorption rate (R~v~) as a function of K^o^~L~ and a~v~. The optimization algorithm used in this study follows a modified Levenberg‐Marquardt method with a trust region approach. The R~v~ predictions from the model are in good agreement with the experimental data, with an average error of 6.5%.